Kaiserslautern - Fachbereich Physik
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Dynamics of Excited Electrons in Copper and Ferromagnetic Transition Metals: Theory and Experiment
(2000)
Both theoretical and experimental results for the dynamics of photoexcited electrons at surfaces of Cu and the ferromagnetic transition metals Fe, Co, and Ni are presented. A model for the dynamics of excited electrons is developed, which is based on the Boltzmann equation and includes effects of photoexcitation, electron-electron scattering, secondary electrons (cascade and Auger electrons), and transport of excited carriers out of the detection region. From this we determine the time-resolved two-photon photoemission (TR-2PPE). Thus a direct comparison of calculated relaxation times with experimental results by means of TR-2PPE becomes possible. The comparison indicates that the magnitudes of the spin-averaged relaxation time t and of the ratio t_up/t_down of majority and minority relaxation times for the different ferromagnetic transition metals result not only from density-of-states effects, but also from different Coulomb matrix elements M. Taking M_Fe > M_Cu > M_Ni = M_Co we get reasonable agreement with experiments.
For the next generation of high data rate magnetic recording above 1 Gbit/s, a better understanding of the switching processes for both recording heads and media will be required. In order to maximize the switch-ing speed for such devices, the magnetization precession after the magnetic field pulse termination needs to be suppressed to a maximum degree. It is demonstrated experimentally for ferrite films that the appropriate adjustment of the field pulse parameters and/or the static applied field may lead to a full suppression of the magnetization precession immediately upon termination of the field pulse. The suppression is explained by taking into account the actual direction of the magnetization with respect to the static field direction at the pulse termination.
Abstract: The recently proposed idea to generate entanglement between photon states via exchange interactions in an ensemble of atoms (J. D. Franson and T. B. Pitman, Phys. Rev. A 60 , 917 (1999) and J. D. Franson et al., (quant- ph/9912121)) is discussed using an S -matix approach. It is shown that if the nonlinear response of the atoms is negligible and no additional atom-atom interactions are present, exchange interactions cannot produce entanglement between photons states in a process that returns the atoms to their initial state. Entanglement generation requires the presence of a nonlinear atomic response or atom-atom interactions.
Abstract: Local field effects on the rate of spontaneous emission and Lamb shift in a dense gas of atoms are discussed taking into account correlations of atomic center-of-mass coordinates. For this the exact retarded propagator in the medium is calculated in independent scattering approximation and employing a virtual-cavity model. The resulting changes of the atomic polarizability lead to modi cations of the medium response which can be of the same order of magnitude but of opposite sign than those due to local field corrections of the dielectric function derived by Morice, Castin, and Dalibard [Phys.Rev.A 51, 3896 (1995)].
Abstract: We identify form-stable coupled excitations of light and matter ("dark-state polaritons") associated with the propagation of quantum fields in Electromagnetically Induced Transparency. The properties of the dark-state polaritons such as the group velocity are determined by the mixing angle between light and matter components and can be controlled by an external coherent field as the pulse propagates. In particular, light pulses can be decelerated and "trapped" in which case their shape and quantum state are mapped onto metastable collective states of matter. Possible applications of this reversible coherent-control technique are discussed.
Abstract: We analyze the above-threshold behavior of a mirrorless parametric oscillator based on resonantly enhanced four wave mixing in a coherently driven dense atomic vapor. It is shown that, in the ideal limit, an arbitrary small flux of pump photons is sufficient to reach the oscillator threshold. We demonstrate that due to the large group velocity delays associated with coherent media, an extremely narrow oscillator linewidth is possible, making a narrow-band source of non-classical radiation feasible.
Abstract: We analyze systematic (classical) and fundamental (quantum) limitations of the sensitivity of optical magnetometers resulting from ac-Stark shifts. We show that incontrast to absorption-based techniques, the signal reduction associated with classical broadening can be compensated in magnetometers based on phase measurements using electromagnetically induced transparency (EIT). However due to ac-Stark associated quantum noise the signal-to-noise ratio of EIT-based magnetometers attains a maximum value at a certain laser intensity. This value is independent on the quantum statistics of the light and defines a standard quantum limit of sensitivity. We demonstrate that an EIT-based optical magnetometer in Faraday configuration is the best candidate to achieve the highest sensitivity of magnetic field detection and give a detailed analysis of such a device.
A simple method of calculating the Wannier-Stark resonances in 2D lattices is suggested. Using this method we calculate the complex Wannier-Stark spectrum for a non-separable 2D potential realized in optical lattices and analyze its general structure. The dependence of the lifetime of Wannier-Stark states on the direction of the static field (relative to the crystallographic axis of the lattice) is briefly discussed.
The paper studies the dynamics of transitions between the levels of a Wannier-Stark ladder induced by a resonant periodic driving. The analysis of the problem is done in terms of resonance quasienergy states, which take into account the metastable character of the Wannier-Stark states. It is shown that the periodic driving creates from a localized Wannier-Stark state an extended Bloch-like state with a spatial length varying in time as ~ t^1/2. Such a state can find applications in the field of atomic optics because it generates a coherent pulsed atomic beam.
The statistics of the resonance widths and the behavior of the survival probability is studied in a particular model of quantum chaotic scattering (a particle in a periodic potential subject to static and time-periodic forces) introduced earlier in Ref. [5,6]. The coarse-grained distribution of the resonance widths is shown to be in good agreement with the prediction of Random Matrix Theory (RMT). The behavior of the survival probability shows, however, some deviation from RMT.